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Multimodal Ultrafast Spectroscopy System Based on a 35 Femtosecond Ti:Sapphire Chirped Pulse Amplification (CPA) Laser

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Multimodal Ultrafast Spectroscopy System Based on a 35 Femtosecond Ti:Sapphire Chirped Pulse Amplification (CPA) Laser

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With technology pushing laser pulse durations into the femtosecond regime1 , the development of methods for timeresolved ultrafast nonlinear spectroscopy to determine the dynamics of atomic and molecular systems seems inevitable. While X-ray crystallography2 and NMR spectroscopy3,4 have provided unprecedented information on the structures of molecules and revealed dynamics in micro-to-millisecond time scales, ultrafast nonlinear spectroscopy serves as a complementary tool for understanding the molecular dynamics on femto- to nanosecond time scales.

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